Temperature‐dependent electromagnetic microwave absorbing characteristics of stretchable polyurethane composite foams with ultra‐wide bandwidth

Publisher:
Wiley
Publication Type:
Journal Article
Citation:
Advanced Engineering Materials, 2022, 24, (7)
Issue Date:
2022-01-01
Full metadata record
With the rapid development of current electronic equipment, electromagnetic microwave absorption (EMA) materials with higher design requirements under special circumstances have attracted great attention. Herein, a flexible polyurethane composite foam assisted by coral-like CNT@Fe3O4/graphene nanocomposites is fabricated by a facile solvothermal and moisture self-foaming method. The composite foam with 15 wt% nanofillers exhibits an outstanding temperature cycle stability with gradually improved EMA performance at elevated temperature and excellent resilience stability with a tensile strength of 4.81 MPa. An enhanced minimum reflection loss (RLmin) of −59.44 dB at 10.38 GHz with a thickness of 2.28 mm is achieved, while the ultrawide absorption bandwidth of 6.09 GHz nearly covers the full X-band. This benefits from interface impedance matching, dielectric and magnetic dual losses, and multiple reflections depending on the interior open microcellular structures. It is expected to become a promising thermally tunable microwave absorber in harsh environments.
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