Confined Sulfur in 3 D MXene/Reduced Graphene Oxide Hybrid Nanosheets for Lithium–Sulfur Battery

Bao, W; Xie, X; Xu, J; Guo, X; Song, J; Wu, W; Su, D; Wang, G

Confined Sulfur in 3 D MXene/Reduced Graphene Oxide Hybrid Nanosheets for Lithium–Sulfur Battery

Bao, W Xie, X

Xu, J Guo, X

Song, J

Wu, W

Su, D

Wang, G

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Publication Type:: Journal Article
Citation:: Chemistry - A European Journal, 2017, 23 (51), pp. 12613 - 12619
Issue Date:: 2017-01-01

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Field	Value	Language
dc.contributor.author	Bao, W	en_US
dc.contributor.author	Xie, X https://orcid.org/0000-0002-8670-8397	en_US
dc.contributor.author	Xu, J	en_US
dc.contributor.author	Guo, X https://orcid.org/0000-0001-7771-0463	en_US
dc.contributor.author	Song, J https://orcid.org/0000-0001-6515-5829	en_US
dc.contributor.author	Wu, W https://orcid.org/0000-0002-3601-9294	en_US
dc.contributor.author	Su, D https://orcid.org/0000-0002-3972-8205	en_US
dc.contributor.author	Wang, G https://orcid.org/0000-0003-4295-8578	en_US
dc.date.issued	2017-01-01	en_US
dc.identifier.citation	Chemistry - A European Journal, 2017, 23 (51), pp. 12613 - 12619	en_US
dc.identifier.issn	0947-6539	en_US
dc.identifier.uri	http://hdl.handle.net/10453/107389
dc.description.abstract	© 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim Three-dimensional metal carbide MXene/reduced graphene oxide hybrid nanosheets are prepared and applied as a cathode host material for lithium–sulfur batteries. The composite cathodes are obtained through a facile and effective two-step liquid-phase impregnation method. Owing to the unique 3 D layer structure and functional 2 D surfaces of MXene and reduced graphene oxide nanosheets for effective trapping of sulfur and lithium polysulfides, the MXene/reduced graphene oxide/sulfur composite cathodes deliver a high initial capacity of 1144.2 mAh g−1 at 0.5 C and a high level of capacity retention of 878.4 mAh g−1 after 300 cycles. It is demonstrated that hybrid metal carbide MXene/reduced graphene oxide nanosheets could be a promising cathode host material for lithium–sulfur batteries.	en_US
dc.relation.ispartof	Chemistry - A European Journal	en_US
dc.relation.isbasedon	10.1002/chem.201702387	en_US
dc.subject.classification	General Chemistry	en_US
dc.title	Confined Sulfur in 3 D MXene/Reduced Graphene Oxide Hybrid Nanosheets for Lithium–Sulfur Battery	en_US
dc.type	Journal Article
utslib.citation.volume	51	en_US
utslib.citation.volume	23	en_US
utslib.for	0303 Macromolecular and Materials Chemistry	en_US
utslib.for	03 Chemical Sciences	en_US
pubs.embargo.period	Not known	en_US
pubs.organisational-group	/University of Technology Sydney
pubs.organisational-group	/University of Technology Sydney/Faculty of Science
pubs.organisational-group	/University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences
pubs.organisational-group	/University of Technology Sydney/Strength - CCET - Centre for Clean Energy Technology
pubs.organisational-group	/University of Technology Sydney/Students
utslib.copyright.status	closed_access
pubs.issue	51	en_US
pubs.publication-status	Published	en_US
pubs.volume	23	en_US

Abstract:

© 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim Three-dimensional metal carbide MXene/reduced graphene oxide hybrid nanosheets are prepared and applied as a cathode host material for lithium–sulfur batteries. The composite cathodes are obtained through a facile and effective two-step liquid-phase impregnation method. Owing to the unique 3 D layer structure and functional 2 D surfaces of MXene and reduced graphene oxide nanosheets for effective trapping of sulfur and lithium polysulfides, the MXene/reduced graphene oxide/sulfur composite cathodes deliver a high initial capacity of 1144.2 mAh g−1 at 0.5 C and a high level of capacity retention of 878.4 mAh g−1 after 300 cycles. It is demonstrated that hybrid metal carbide MXene/reduced graphene oxide nanosheets could be a promising cathode host material for lithium–sulfur batteries.

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http://hdl.handle.net/10453/107389