Enhanced Emission from Interlayer Excitons Coupled to Plasmonic Gap Cavities.

Tran, TN; Kim, S; White, SJU; Nguyen, MAP; Xiao, L; Strauf, S; Yang, T; Aharonovich, I; Xu, Z-Q

Enhanced Emission from Interlayer Excitons Coupled to Plasmonic Gap Cavities.

Tran, TN Kim, S

White, SJU Nguyen, MAP Xiao, L Strauf, S Yang, T

Aharonovich, I

Xu, Z-Q

Permalink

Publisher:: Wiley
Publication Type:: Journal Article
Citation:: Small, 2021, 17, (45), pp. 1-7
Issue Date:: 2021-11

Closed Access

	Filename	Description	Size
	Small - 2021 - Tran - Enhanced Emission from Interlayer Excitons Coupled to Plasmonic Gap Cavities.pdf		1.15 MB	Adobe PDF	View/Open

Copyright Clearance Process

Recently Added
In Progress
Closed Access

This item is closed access and not available.

Full metadata record

Field	Value	Language
dc.contributor.author	Tran, TN
dc.contributor.author	Kim, S https://orcid.org/0000-0001-9836-3608
dc.contributor.author	White, SJU
dc.contributor.author	Nguyen, MAP
dc.contributor.author	Xiao, L
dc.contributor.author	Strauf, S
dc.contributor.author	Yang, T https://orcid.org/0000-0002-8683-2072
dc.contributor.author	Aharonovich, I https://orcid.org/0000-0003-4304-3935
dc.contributor.author	Xu, Z-Q
dc.date.accessioned	2022-01-17T02:38:14Z
dc.date.available	2022-01-17T02:38:14Z
dc.date.issued	2021-11
dc.identifier.citation	Small, 2021, 17, (45), pp. 1-7
dc.identifier.issn	1613-6810
dc.identifier.issn	1613-6829
dc.identifier.uri	http://hdl.handle.net/10453/153199
dc.description.abstract	The emergence of interlayer excitons (IEs) from atomic layered transition metal dichalcogenides (TMDCs) heterostructures has drawn tremendous attention due to their unique and exotic optoelectronic properties. Coupling the IEs into optical cavities provides distinctive electromagnetic environments which plays an important role in controlling multiple optical processes such as optical nonlinear generation or photoluminescence enhancement. Here, the integration of IEs in TMDCs into plasmonic nanocavities based on a nanocube on a metallic mirror is reported. Spectroscopic studies reveal an order of magnitude enhancement of the IE at room temperature and a 5-time enhancement in fluorescence at cryogenic temperatures. Cavity modeling reveals that the enhancement of the emission is attributed to both increased excitation efficiency and Purcell effect from the cavity. The results show a novel method to control the excitonic processes in TMDC heterostructures to build high performance photonics and optoelectronics devices.
dc.format	Print-Electronic
dc.language	eng
dc.publisher	Wiley
dc.relation	http://purl.org/au-research/grants/arc/CE200100010
dc.relation.ispartof	Small
dc.relation.isbasedon	10.1002/smll.202103994
dc.rights	info:eu-repo/semantics/closedAccess
dc.subject.classification	Nanoscience & Nanotechnology
dc.title	Enhanced Emission from Interlayer Excitons Coupled to Plasmonic Gap Cavities.
dc.type	Journal Article
utslib.citation.volume	17
utslib.location.activity	Germany
pubs.organisational-group	/University of Technology Sydney
pubs.organisational-group	/University of Technology Sydney/Faculty of Science
pubs.organisational-group	/University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences
utslib.copyright.status	closed_access	*
pubs.consider-herdc	false
dc.date.updated	2022-01-17T02:38:13Z
pubs.issue	45
pubs.publication-status	Published
pubs.volume	17
utslib.citation.issue	45

Abstract:

The emergence of interlayer excitons (IEs) from atomic layered transition metal dichalcogenides (TMDCs) heterostructures has drawn tremendous attention due to their unique and exotic optoelectronic properties. Coupling the IEs into optical cavities provides distinctive electromagnetic environments which plays an important role in controlling multiple optical processes such as optical nonlinear generation or photoluminescence enhancement. Here, the integration of IEs in TMDCs into plasmonic nanocavities based on a nanocube on a metallic mirror is reported. Spectroscopic studies reveal an order of magnitude enhancement of the IE at room temperature and a 5-time enhancement in fluorescence at cryogenic temperatures. Cavity modeling reveals that the enhancement of the emission is attributed to both increased excitation efficiency and Purcell effect from the cavity. The results show a novel method to control the excitonic processes in TMDC heterostructures to build high performance photonics and optoelectronics devices.

Please use this identifier to cite or link to this item:

http://hdl.handle.net/10453/153199