Tailoring pores in graphene-based materials: from generation to applications
- Publisher:
- Royal Society of Chemistry
- Publication Type:
- Journal Article
- Citation:
- Journal of Materials Chemistry A, 2017, 5, (32), pp. 16537-16558
- Issue Date:
- 2017-08-28
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Combining the merits from both porous material and graphene, porous graphene-based materials have
received significant attention due to their unique porous structures, large surface areas and prominent
electrical conductivity. The access and tuning of both the in-plane pores of a monolayer graphene and the
interlayer spacing (interlayered pores) of multilayered graphene-based materials offer additional selective
mechanisms. These extraordinary properties enable porous graphene-based materials to serve as critical
components in molecular separation, including water desalination, gas separation and bioseparation, and
electrochemical energy storage, such as supercapacitors, lithium–O2/ion/sulfur batteries and fuel cells. The
state-of-the-art pore-fabrication methods as well as the interlayered pores tuning approach for graphene-based materials are summarized. The insights between structures, properties and the broad applications of
these materials are reviewed and discussed. The remaining challenges and future perspectives of porous
graphene-based materials for wide implementations are provided.
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