Efficient FRET process between CsPbBr<inf>3</inf> quantum dots and RhB dye molecules by pressure regulation

Gao, YS; Xu, YL; Yang, TS; Wang, HG; Mu, HF; Tan, XM; Yang, CL; Wang, K; Li, ZG; Xu, QF

Efficient FRET process between CsPbBr<inf>3</inf> quantum dots and RhB dye molecules by pressure regulation

Gao, YS Xu, YL Yang, TS Wang, HG Mu, HF Tan, XM Yang, CL Wang, K Li, ZG Xu, QF

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Publisher:: AIP Publishing
Publication Type:: Journal Article
Citation:: Applied Physics Letters, 2023, 123, (21), pp. 212102
Issue Date:: 2023-11-20

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Field	Value	Language
dc.contributor.author	Gao, YS
dc.contributor.author	Xu, YL
dc.contributor.author	Yang, TS
dc.contributor.author	Wang, HG
dc.contributor.author	Mu, HF
dc.contributor.author	Tan, XM
dc.contributor.author	Yang, CL
dc.contributor.author	Wang, K
dc.contributor.author	Li, ZG
dc.contributor.author	Xu, QF
dc.date.accessioned	2024-04-23T22:46:21Z
dc.date.available	2024-04-23T22:46:21Z
dc.date.issued	2023-11-20
dc.identifier.citation	Applied Physics Letters, 2023, 123, (21), pp. 212102
dc.identifier.issn	0003-6951
dc.identifier.issn	1077-3118
dc.identifier.uri	http://hdl.handle.net/10453/178307
dc.description.abstract	Fluorescence resonance energy transfer (FRET) based on quantum dots (QDs) and dye molecules have great application potential in biochemical fields. How to achieve an efficient energy transfer process has become an important research topic. Pressure can be used to regulate the energy transfer process, but its regulation on metal halide perovskite systems is rarely reported. Herein, the efficient FRET process between CsPbBr3 QDs and Rhodamine B (RhB) molecules under high pressure is investigated. Upon compression to 1.3 GPa, the FRET rate of the CsPbBr3-RhB composite reaches 0.21 ns−1 and the FRET efficiency is improved from 12.4% to 62.4%, due to enhanced spectral overlap and shortened minimum distance between CsPbBr3 QDs and RhB molecules. This study provides a strategy for achieving efficient FRET research and further promotes the development of applications based on halide perovskite molecular systems.
dc.language	en
dc.publisher	AIP Publishing
dc.relation.ispartof	Applied Physics Letters
dc.relation.isbasedon	10.1063/5.0176861
dc.rights	info:eu-repo/semantics/embargoedAccess
dc.subject	02 Physical Sciences, 09 Engineering, 10 Technology
dc.subject.classification	Applied Physics
dc.subject.classification	40 Engineering
dc.subject.classification	51 Physical sciences
dc.title	Efficient FRET process between CsPbBr<inf>3</inf> quantum dots and RhB dye molecules by pressure regulation
dc.type	Journal Article
utslib.citation.volume	123
utslib.for	02 Physical Sciences
utslib.for	09 Engineering
utslib.for	10 Technology
pubs.organisational-group	University of Technology Sydney
pubs.organisational-group	University of Technology Sydney/Faculty of Science
pubs.organisational-group	University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences
utslib.copyright.status	embargoed	*
utslib.copyright.embargo	2024-11-02T00:00:00+1000Z
dc.date.updated	2024-04-23T22:46:20Z
pubs.issue	21
pubs.publication-status	Published
pubs.volume	123
utslib.citation.issue	21

Abstract:

Fluorescence resonance energy transfer (FRET) based on quantum dots (QDs) and dye molecules have great application potential in biochemical fields. How to achieve an efficient energy transfer process has become an important research topic. Pressure can be used to regulate the energy transfer process, but its regulation on metal halide perovskite systems is rarely reported. Herein, the efficient FRET process between CsPbBr3 QDs and Rhodamine B (RhB) molecules under high pressure is investigated. Upon compression to 1.3 GPa, the FRET rate of the CsPbBr3-RhB composite reaches 0.21 ns−1 and the FRET efficiency is improved from 12.4% to 62.4%, due to enhanced spectral overlap and shortened minimum distance between CsPbBr3 QDs and RhB molecules. This study provides a strategy for achieving efficient FRET research and further promotes the development of applications based on halide perovskite molecular systems.

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http://hdl.handle.net/10453/178307