Progress and Perspective of High-Entropy Strategy Applied in Layered Transition Metal Oxide Cathode Materials for High-Energy and Long Cycle Life Sodium-Ion Batteries

Wang, L; Wang, L; Wang, H; Dong, H; Sun, W; Lv, LP; Yang, C; Xiao, Y; Wu, F; Wang, Y; Chou, S; Sun, B; Wang, G; Chen, S

Progress and Perspective of High-Entropy Strategy Applied in Layered Transition Metal Oxide Cathode Materials for High-Energy and Long Cycle Life Sodium-Ion Batteries

Wang, L Wang, L Wang, H Dong, H Sun, W Lv, LP Yang, C Xiao, Y Wu, F Wang, Y Chou, S Sun, B

Wang, G Chen, S

Permalink

Publisher:: WILEY-V C H VERLAG GMBH
Publication Type:: Journal Article
Citation:: Advanced Functional Materials, 2024
Issue Date:: 2024-01-01

Closed Access

	Filename	Description	Size
	Adv Funct Materials - 2024 - Wang - Progress and Perspective of High‐Entropy Strategy Applied in Layered Transition Metal.pdf	Accepted version	6.69 MB		View/Open

Copyright Clearance Process

Recently Added
In Progress
Closed Access

This item is closed access and not available.

Full metadata record

Field	Value	Language
dc.contributor.author	Wang, L
dc.contributor.author	Wang, L
dc.contributor.author	Wang, H
dc.contributor.author	Dong, H
dc.contributor.author	Sun, W
dc.contributor.author	Lv, LP
dc.contributor.author	Yang, C
dc.contributor.author	Xiao, Y
dc.contributor.author	Wu, F
dc.contributor.author	Wang, Y
dc.contributor.author	Chou, S
dc.contributor.author	Sun, B https://orcid.org/0000-0002-4365-486X
dc.contributor.author	Wang, G
dc.contributor.author	Chen, S
dc.date.accessioned	2025-01-30T06:30:07Z
dc.date.available	2025-01-30T06:30:07Z
dc.date.issued	2024-01-01
dc.identifier.citation	Advanced Functional Materials, 2024
dc.identifier.issn	1616-301X
dc.identifier.issn	1616-3028
dc.identifier.uri	http://hdl.handle.net/10453/184676
dc.description.abstract	Layered transition metal oxide (LTMO) cathode materials of sodium-ion batteries (SIBs) have shown great potential in large-scale energy storage applications owing to their distinctive periodic layered structure and 2D ion diffusion channels. However, several challenges have hindered their widespread application, including phase transition complexities, interface instability, and susceptibility to air exposure. Fortunately, an impactful solution has emerged in the form of a high-entropy doping strategy employed in energy storage research. Through the implementation of high-entropy doping, LTMOs can overcome the aforementioned limitations, thereby elevating LTMO materials to a highly competitive and attractive option for next-generation cathodes of SIBs. Thus, a comprehensive overview of the origins, definition, and characteristics of high-entropy doping is provided. Additionally, the challenges associated with LTMOs in SIBs are explored, and discussed various modification methods to address these challenges. This review places significant emphasis on conducting a thorough analysis of the research advancements about high-entropy LTMOs utilized in SIBs. Furthermore, a meticulous assessment of the future development trajectory is undertaken, heralding valuable research insights for the design and synthesis of advanced energy storage materials.
dc.language	English
dc.publisher	WILEY-V C H VERLAG GMBH
dc.relation	http://purl.org/au-research/grants/arc/FT220100561
dc.relation.ispartof	Advanced Functional Materials
dc.relation.isbasedon	10.1002/adfm.202417258
dc.rights	info:eu-repo/semantics/closedAccess
dc.subject	02 Physical Sciences, 03 Chemical Sciences, 09 Engineering
dc.subject.classification	Materials
dc.subject.classification	34 Chemical sciences
dc.subject.classification	40 Engineering
dc.subject.classification	51 Physical sciences
dc.title	Progress and Perspective of High-Entropy Strategy Applied in Layered Transition Metal Oxide Cathode Materials for High-Energy and Long Cycle Life Sodium-Ion Batteries
dc.type	Journal Article
utslib.for	02 Physical Sciences
utslib.for	03 Chemical Sciences
utslib.for	09 Engineering
pubs.organisational-group	University of Technology Sydney
pubs.organisational-group	University of Technology Sydney/Faculty of Science
pubs.organisational-group	University of Technology Sydney/Faculty of Science/School of Mathematical and Physical Sciences
pubs.organisational-group	University of Technology Sydney/UTS Groups
pubs.organisational-group	University of Technology Sydney/UTS Groups/Centre for Clean Energy Technology (CCET)
utslib.copyright.status	closed_access	*
dc.date.updated	2025-01-30T06:30:05Z
pubs.publication-status	Published

Abstract:

Layered transition metal oxide (LTMO) cathode materials of sodium-ion batteries (SIBs) have shown great potential in large-scale energy storage applications owing to their distinctive periodic layered structure and 2D ion diffusion channels. However, several challenges have hindered their widespread application, including phase transition complexities, interface instability, and susceptibility to air exposure. Fortunately, an impactful solution has emerged in the form of a high-entropy doping strategy employed in energy storage research. Through the implementation of high-entropy doping, LTMOs can overcome the aforementioned limitations, thereby elevating LTMO materials to a highly competitive and attractive option for next-generation cathodes of SIBs. Thus, a comprehensive overview of the origins, definition, and characteristics of high-entropy doping is provided. Additionally, the challenges associated with LTMOs in SIBs are explored, and discussed various modification methods to address these challenges. This review places significant emphasis on conducting a thorough analysis of the research advancements about high-entropy LTMOs utilized in SIBs. Furthermore, a meticulous assessment of the future development trajectory is undertaken, heralding valuable research insights for the design and synthesis of advanced energy storage materials.

Please use this identifier to cite or link to this item:

http://hdl.handle.net/10453/184676